Corrosion Damage Mechanisms of TiO₂ Cold-Sprayed Coatings

• Autorzy: Lachowicz Marzena , Winnicki Marcin

Identyfikatory

DOI

10.24425/amm.2022.139691

• Języki publikacji: EN

Abstrakty

EN

Cold spraying as a low-temperature coating deposition method is intended for thermally sensitive materials. Due to its precise temperature control, it limits the formation of structural defects, and can therefore be easily applied to spray corrosion protective coatings made from metal or metal-ceramic powders. However, the formation of pure ceramic coatings with the use of cold spraying is still not so common. Titanium dioxide is one of the most interesting ceramics due to its photocatalytic properties. Nevertheless, these types of coating materials usually work in a corrosion favoring humid atmosphere. In the presented paper, amorphous TiO₂ powder was deposited onto aluminum alloys and steel substrates and then submitted to potentiodynamic corrosion tests in a 3.5 wt.% NaCl solution. The as-sprayed coating showed phase transition from amorphous TiO₂ to anatase, and also revealed porosity. As a result, electrolytes penetrated the coating and caused undercoating corrosion in the tested environment of an aqueous NaCl solution. The analysis of the potentiodynamic curves showed that the presence of the coating decreased corrosion potential on both substrates. It arose from the mixed phases of TiO₂, which consisted of photocathode - amorphous material and photoanode - crystalline anatase. The phase mixture induced the galvanic corrosion of metallic substrates in the presence of electrolytes. Moreover, pitting-like corrosion and coating delamination were detected in aluminium alloy and steel samples, respectively. Finally, the corrosion mechanism of the titanium dioxide coatings was characterized and described.

Słowa kluczowe

EN

titanium dioxide; cold-sprayed coatings; potentiodynamic polarization test; aluminum alloys; structural steel

• Wydawca: Institute of Metallurgy and Materials Science of Polish Academy of Sciences ; Committee of Materials Engineering and Metallurgy of Polish Academy of Sciences
• Czasopismo: Archives of Metallurgy and Materials
• Rocznik: 2022
• Tom: Vol. 67, iss. 3
• Strony: 975--985
• Opis fizyczny: Bibliogr. 71 poz., fot., rys., tab.

Twórcy

autor

Lachowicz Marzena

• Wrocław University of Science and Technology, Department of Metal Forming, Welding and Metrology, 5 Lukasiewicza Str., 50-371 Wroclaw, Poland

• https://orcid.org/0000-0002-4959-2970

autor

Winnicki Marcin

• Wrocław University of Science and Technology, Department of Metal Forming, Welding and Metrology, 5 Lukasiewicza Str., 50-371 Wroclaw, Poland

• https://orcid.org/0000-0003-2766-116X

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Uwagi

1. This research was funded by Polish National Science Centre under the Contract No. 2016/23/D/ST8/00675 (Project title: The mechanism of joining submicron ceramic particles in cold spraying process).

2. Opracowanie rekordu ze środków MNiSW, umowa nr SONP/SP/546092/2022 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2024).