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Tytuł artykułu

Mechanical flexibility and electrical reliability of ZnO-Al thin films on polymer substrates under different external deformation

Identyfikatory
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
Aluminum-doped zinc oxide (AZO) films have emerged as promising transparent electrodes for various optoelectronic applications due to their superior transparency, electrical conductivity, and cost-effectiveness compared to indium tin oxide (ITO). Despite their widespread use, investigations into the electromechanical properties of AZO films, especially under various mechanical deformations, remain limited. This study employs RF magnetron sputtering to deposit AZO films on polyethylene naphthalate (PEN) substrates and explores their mechanical behavior through uniaxial tensile fragmentation and bending tests, coupled with in-situ optical microscopy. Changes in electrical resistance of AZO films were monitored in situ during deformation. Fatigue behavior was examined to further understand mechanical failure, and SEM was used for surface characterization. A critical strain of about 3.1 percent was detected during uniaxial tensile testing, marking the onset of cracks in AZO-coated PEN. In contrast to thicker films, thinner films demonstrated improved stretchability beyond the initiation of crack onset strain. Tension and compression bending tests revealed that the material has excellent bendability, as shown by its critical radii of 5.4 mm and 3.9 mm, respectively. The bending reliability of AZO films under compression was found to be superior than that under tension. Bending fatigue experiments demonstrated that AZO films could withstand cyclic stress without experiencing noticeable cracks after 100 cycles and with very minor resistance change. This study contributes to the creation of more reliable and optimized flexible optoelectronic devices by giving substantial quantitative data on the performance of AZO films when exposed to mechanical stress.
Rocznik
Strony
32--45
Opis fizyczny
Bibliogr. 32 poz., rys., wykr.
Twórcy
  • University of Duhok, Department of Physics, Zakho way, Duhok, Iraq
  • University of Birmingham, School of Metallurgy and Materials, Edgbaston, Birmingham, B15 2TT, United Kingdom
Bibliografia
  • 1. H.-K. Kim, J.-W. Lim, Flexible IZO/Ag/IZO/Ag multilayer electrode grown on a polyethylene terephthalate substrate using roll-to-roll sputtering, Nanoscale Research Letters. 7 (2012) 67.
  • 2. Q. Xu, W. Shen, Q. Huang, Y. Yang, R. Tan, K. Zhu, N. Dai, W. Song, Flexible transparent conductive films on PET substrates with an AZO/AgNW/AZO sandwich structure, Journal of Materials Chemistry C. 2 (2014) 3750.
  • 3. X. Li, P. Li, Z. Wu, D. Luo, H.-Y. Yu, Z.-H. Lu, Review and perspective of materials for flexible solar cells, Materials Reports: Energy. 1 (2021) 100001.
  • 4. S.-Y. Chang, Y.-C. Hsiao, Y.-C. Huang, Preparation and mechanical properties of aluminum-doped zinc oxide transparent conducting films, Surface and Coatings Technology. 202 (2008) 5416–5420.
  • 5. C.Y. Peng, M.M. Hamasha, D. Vanhart, S. Lu, C.R. Westgate, Electrical and optical degradation studies on AZO thin films under cyclic bending conditions, IEEE Transactions on Device and Materials Reliability. 13 (2013) 236–244.
  • 6. G.M. Wu, Y.F. Chen, H.C. Lu, Aluminum-Doped Zinc Oxide Thin Films Prepared by Sol-Gel and RF Magnetron Sputtering, 120 (2011) 149–152.
  • 7. S. Fernández, a. Martínez-Steele, J.J. Gandía, F.B. Naranjo, Radio frequency sputter deposition of high-quality conductive and transparent ZnO:Al films on polymer substrates for thin film solar cells applications, Thin Solid Films. 517 (2009) 3152–3156..
  • 8. K.A. Sierros, D.S. Hecht, D.A. Banerjee, N.J. Morris, L. Hu, G.C. Irvin, R.S. Lee, D.R. Cairns, Durable transparent carbon nanotube films for flexible device components, Thin Solid Films. 518 (2010) 6977–6983.
  • 9. M.M. Hamasha, K. Alzoubi, S. Lu, Behavior of sputtered indium-tin-oxide thin film on poly-ethylene terephthalate substrate under stretching, IEEE/OSA Journal of Display Technology. 7 (2011) 426–433.
  • 10. C.-Y. Lim, J.-K. Park, Y.-H. Kim, J.-I. Han, Mechanical and Electrical Stability Indium-Tin-Oxide Coated Polymer Substrates under Continuous Bending Stress Condition, Journal of International Council on Electrical Engineering. 2 (2012) 237–241.
  • 11. J.L. Ni, X.F. Zhu, Z.L. Pei, J. Gong, C. Sun, G.P. Zhang, Comparative investigation of fracture behaviour of aluminium-doped ZnO films on a flexible substrate, Journal of Physics D: Applied Physics. 42 (2009) 175404(7pp).
  • 12. C.Y. Peng, H. Sudarsanam, M.M. Hamasha, S. Lu, T.P. Dhakal, C.R. Westgate, Performance of aluminum-doped zinc oxide thin films under bending fatigue conditions, 2012 IEEE Long Island Systems, Applications and Technology Conference, LISAT 2012. (2012).
  • 13. Z. Chen, B. Cotterell, W. Wang, E. Guenther, S. Chua, A mechanical assessment of flexible optoelectronic devices, Thin Solid Films. 394 (2001) 202–206.
  • 14. D.W. Mohammed, R. Waddingham, A.J. Flewitt, K.A. Sierros, J. Bowen, S.N. Kukureka, Mechanical properties of amorphous indium-gallium-zinc oxide thin films on compliant substrates for flexible optoelectronic devices, Thin Solid Films. 594 (2015) 197–204.
  • 15. D.W. Mohammed, Mechanical and electro-mechanical reliability of transparent oxide thin films for flexible electronics applications, PhD thesis, University of Birmingham, 2016. https://doi.org/https://etheses.bham.ac.uk//id/eprint/7997/1/Mohammed17PhD.pdf.
  • 16. Z. Chen, A mechanical assessment of flexible optoelectronic devices, Thin Solid Films. 394 (2001) 201–205.
  • 17. Q. Guan, J. Laven, P.C.P. Bouten, G. De With, Mechanical failure of brittle thin films on polymers during bending by two-point rotation, Thin Solid Films. 611 (2016) 107–116.
  • 18. M.J. Cordill, P. Kreiml, H. Köstenbauer, C. Mitterer, A comparison of 90◦ bending for foldable electronics, Coatings. 14 (2024) 98.
  • 19. D.W. Mohammed, R.B. Ameen, K.A. Sierros, J. Bowen, S.N. Kukureka, Twisting fatigue in multilayer films of Ag-alloy with indium tin oxide on polyethylene terephthalate for flexible electronics devices, Thin Solid Films. 645 (2018) 241–252..
  • 20. G.A. Potoczny, Electro-Mechanical Behaviour of Indium Tin Oxide Coated Polymer Substrates for Flexible Electronics, (2012).
  • 21. A.A. Abdallah, P.C.P. Bouten, J.M.J. den Toonder, G. De With, Buckle initiation and delamination of patterned ITO layers on a polymer substrate, Surface and Coatings Technology. 205 (2011) 3103–3111.
  • 22. Z. Zhao, H. Fu, R. Tang, B. Zhang, Y. Chen, J. Jiang, Failure mechanisms in flexible electronics, International Journal of Smart and Nano Materials. 14 (2023) 510–565.
  • 23. T.S. Bejitual, D. Compton, K.A. Sierros, D.R. Cairns, S.N. Kukureka, Electromechanical reliability of flexible transparent electrodes during and after exposure to acrylic acid, Thin Solid Films. 528 (2013) 229–236.
  • 24. S. Frank, U. a. Handge, S. Olliges, R. Spolenak, The relationship between thin film fragmentation and buckle formation: Synchrotron-based in situ studies and two-dimensional stress analysis, Acta Materialia. 57 (2009) 1442–1453.
  • 25. L. Rebouta, L. Rubio Pena, C. Oliveira, S. Lanceros-Mendez, C.J. Tavares, E. Alves, Strain dependence electrical resistance and cohesive strength of ITO thin films deposited on electroactive polymer, Thin Solid Films. 518 (2010) 4525–4528.
  • 26. M. J. Cordill, Kreiml, P., C. Mitterer, Materials Engineering for Flexible Metallic Thin Film Applications, Materials. 15 (2022) 1–25.
  • 27. J. Zhou, X. Zhang, X. Zhang, W. Zhang, J. Li, Y. Chen, H. Liu, Y. Yan, Mechanical Properties of Tensile Cracking in Indium Tin Oxide Films on Polycarbonate Substrates, Coatings. 12 (2022) 1–12.
  • 28. D. Tsubone, T. Hasebe, A. Kamijo, A. Hotta, Fracture mechanics of diamond-like carbon (DLC) films coated on flexible polymer substrates, Surface and Coatings Technology. 201 (2007) 6423–6430.
  • 29. D.R. Cairns, R.P. Witte, D.K. Sparacin, S.M. Sachsman, D.C. Paine, G.P. Crawford, R.R. Newton, Strain-dependent electrical resistance of tin-doped indium oxide on polymer substrates, Applied Physics Letters. 76 (2000) 1425.
  • 30. K. Sierros, N.J. Morris, S.N. Kukureka, D.R. Cairns, Dry and wet sliding wear of ITO-coated PET components used in flexible optoelectronic applications, Wear. 267 (2009) 625–631.
  • 31. J.I. Han, Stability of Externally Deformed ITO Films, in: G.P. Crawford (Ed.), Flexible Flat Panel Displays, John Wiley & Sons Ltd, Chichester, 2005: pp. 121–132.
  • 32. Y. Zhi-nong, X. Fan, L. Yu-qiong, X. Wei, The electrical stabilities of flexible ITO thin films on buffer layer coated PET, Optics Info Base Conference Papers. (2008) 3–5.
Uwagi
Opracowanie rekordu ze środków MNiSW, umowa nr SONP/SP/546092/2022 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2024).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-3630e001-6398-4bd1-bdf3-9b7f792be3a2
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