Decolorization Kinetics of Acid Azo Dye and Basic Thiazine Dye in Aqueous Solution by UV/H2O2 and UV/Fenton: Effects of Operational Parameters

• Autorzy: Baffoun A. , El Ghali A. , Hachani I.

Identyfikatory

DOI

10.1515/aut-2016-0031

• Języki publikacji: EN

Abstrakty

EN

The photochemical decolorization of two dyes, namely Acid Yellow 54 and Basic Blue 9, was studied using the UV/H2O2 and UV/Fenton processes. The effects of the amount of H2O2 and FeSO4 as well as the initial pH solution on decolorization kinetics of both the dyes were investigated. The pseudo-first order kinetic model was applied to predict the decolorization of the selected dyes at the different operational conditions and results showed that this model fitted very well with the experimental data. The obtained results also showed the efficiency of UV/Fenton process to quickly degrade aqueous effluents polluted by Acid Yellow 54 and Basic Blue 9 compared to the UV/H2O2 process.

Słowa kluczowe

EN

advanced oxidation processes; AOP; decolorization; UV/H2O2; UV-Fenton; acid dye; basic dye

PL

procesy zaawansowanego utleniania; odbarwianie; UV/H2O2; UV-Fenton; barwnik kwasowy; barwnik zasadowy

• Wydawca: Lodz University of Technology, Faculty of Material Technologies and Textile Design
• Czasopismo: Autex Research Journal
• Rocznik: 2017
• Tom: Vol. 17, no. 1
• Strony: 85--94
• Opis fizyczny: Bibliogr. 28 poz.

Twórcy

autor

Baffoun A.

• Textile Department, National Engineering School of Monastir, Monastir University, Tunisia Textile Materials and Processes Research Unit MPTex, National Engineering School of Monastir -University of Monastir, Tunisia

autor

El Ghali A.

• Textile Department, National Engineering School of Monastir, Monastir University, Tunisia Laboratory of Advanced Materials and Interfaces (LAMI), Faculty of Sciences of Monastir, Monastir University, Tunisia

autor

Hachani I.

• Textile Department, National Engineering School of Monastir, Monastir University, Tunisia

Bibliografia

• [1] Alinsafi A, Da Motta M, Le Bonté S, Pons M N, Benhammou A. (2006). Effect of variability on the treatment of textile dyeing wastewater by activated sludge. Dyes and Pigments, 69, 31-39.
• [2] El Ghali A, Baouabb M H, Roudesli M S. (2011). Preparation, characterization and application of a [copper (II)/ethylenediamine–cotton] complex for the removal of AB25 from aqueous solution in a laboratory scale column. Chemical Engineering Journal, 174, 18-26.
• [3] Rauf M A, Shehadi I A, Hassan W W. (2007). Studies on the removal of Neutral Red on sand from aqueous solution and its kinetics behavior. Dyes and Pigments, 75, 723-726.
• [4] Hameed B H, Din A T M, Ahmad A L. (2007). Adsorption of methylene blue onto bamboo-based activated carbon: Kinetics and equilibrium studies. Journal of Hazardous Materials, 14, 819-825.
• [5] Ahmad A L, Puasa S W. (2007). Reactive dyes decolourization from an aqueous solution by combined coagulation/micellar-enhanced ultrafiltration process. Chemical Engineering Journal, 132, 257-265.
• [6] Baran W, Adamek E, Makowski A. (2008). The influence of selected parameters on the photocatalytic degradation of azo-dyes in the presence of TiO2 aqueous suspension. Chemical Engineering Journal, 145, 242–248.
• [7] Ince NH, Gönenc DT. (1997). Treatability of a textile azo dye by UV/H2O2. Environmental Technology, 18, 179 - 185.
• [8] Arslan I, Balcioglu I A, Bahnemann D W. (2000). Advanced chemical oxidation of reactive dyes in simulated dye house effluents by ferrioxalate-Fenton/UV-A and TiO2/UV-A processes. Dyes and Pigments, 47, 2007-2018.
• [9] Alnuoimi M M, Rauf M A, Ashraf S S. (2007). Comparative decolorization study of Neutral Red by different oxidative processes. Dyes and Pigments, 72, 367-371.
• [10] Neamtu M, Siminiceanu I, Yediler A, Kettrup A. (2002). Kinetics of decolorization and mineralization of reactive azo dyes in aqueous solution by the UV/H2O2 oxidation. Dyes and Pigments, 53, 93-99.
• [11] Ince N.H, Stefan M.I, Bolton J.R. (1997). UV/H2O2 degradation and toxicity reduction of textile azo dyes: remazol Black-B, a case study. Journal of Advanced Oxidation Technology, 2, 442-448.
• [12] Namboodri C.G, Walsh W.K. (1996). Ultraviolet light/hydrogen peroxide system for decolourizing spent reactive dyebath waste water. American Dyestuff Report, 15-25.
• [13] Aleboyeh A, Moussa Y, Aleboyeh H, (2005). The effect of operational parameters on UV/H2O2 decolourisation of Acid Blue 74. Dyes and Pigments, 66, 129-134
• [14] Rauf M A, Marzouki N, Bahadir K. Korbahti. (2008). Photolytic decolorization of Rose Bengal by UV/H2O2 and data optimization using response surface method. Journal of Hazardous Materials, 159, 602-609.
• [15] Ince N.H, Gönenc D.T. (1997). Treatability of a textile azo dye by UV/H2O2. Environmental Technology, 18, 179-185.
• [16] Galindo C, Jacques P, Kalt A. (1999). Total mineralization of an azo dye (acid orange 7) by UV/H2O2 oxidation. Journal of Advanced Oxidation Technology, 1, 160-169.
• [17] Braun A.M, Maurette M.T, Oliveros E. (1991). Photochemical technology. Chichester. Wiley.
• [18] Chu W. (2001). Modelling the quantum yields of herbicide 2,4-D decay in UV/H2O2 process. Chemosphere, 44, 935-941.
• [19] Fenton H J H. (1894). Oxidation of tartaric acid in the presence of iron. Journal of Chemical Society, 6, 899-910.
• [20] Bandeara .J, Marrison.C, Kiwi.J, Pulgarin.C, Pevinger.P. (1996). Degradation of concentrated solutions of Orange II. Kinetics and quantum yield for sunlight induced reactions via Fenton type reagents. Journal of Photochemistry and Photobiology A: Chemistry, 99, 57-66.
• [21] Nedoloujko.A, Kiwi.J. (1997). Parameters affecting the homogeneous and heterogeneous degradation of quinoline solutions in lignt activated processes. Journal of Photochemistry and Photobiology A: Chemistry, 110, 149-157.
• [22] Sykora.J, Pado.M, Tatarko.M, Izakovic.M. (1997). Homogeneous photo-oxidation of phenols: influence of metals. Journal of Photochemistry and Photobiology A: Chemistry, 110, 167-175.
• [23] Zuo.Y, Holgne.J. (1992). Formation of hydrogen peroxide and depletion of oxalic acid in atmospheric water by photolysis of ironIII oxalato complexes. Environmental. Science Technology, 26, 1014-1022.
• [24] David.F, David.P.G,. (1976). Photoredox chemistry of iron(III) chloride and iron(III) perchlorate in aqueous media: A comparative study. Journal of Physical Chemistry, 80, 579-583.
• [25] Bigda R J. (1995). Consider Fenton’s chemistry for wastewater treatment. Chemical Engineering Progress, 91, 62-66.
• [26] Muruganandham M., Swaminatham M. (2004). Decolourisation of Reactive Orange 4 by Fenton and Photo-Fenton oxidation technology. Dyes and Pigments, 63, 315-321.
• [27] Walling C. (1975). Fenton’s reagent revisited. Accounts of Chemical Research, 8, 125-131.
• [28] Fernandez J, Bandara J, Lopez A, Buffar Ph, Kiwi J. (1999). Photo-assisted Fenton degradation of nonbiodegradable azo dye (Orange II) in Fe-free solutions mediated by cation transfer membranes. Langmuir, 15(1), 185-192.