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A Prefatory Sustainability Assessment of One-Part Geopolymers

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Języki publikacji
EN
Abstrakty
EN
This study investigated the sustainability aspect of the fly ash (FA)-based one-part geopolymers (OPGs) with various combinations and amount of alkali activators (AA). The three groups of OPG were: the M-OPG activated with solely sodium metasilicate-anhydrous (Na2SiO3), the MH-OPG with Na2SiO3 and sodium hydroxide (NaOH), and the MC-OPG with Na2SiO3 and sodium carbonate (Na2CO3). The compressive strength, embodied carbon, embodied carbon index, embodied energy and embodied energy index were identified. Test result shows that the M-OPG and MC-OPG with the AA/FA ratio of 0.20 attained 83 MPa and 75 MPa of compressive strengths, respectively. The MH-OPG with AA/FA ratio of 0.15 attained 72 MPa of compressive strength. The embodied carbon and embodied energy of the OPGs were mainly contributed by the Na2SiO3-anhydrous. The values were lowered when the Na2SiO3-anhydrous were partially substituted with NaOH or Na2CO3. Increasing the AA content increased the embodied carbon and energy. The embodied carbon index (3.80 kg CO2/m3/MPa) and embodied energy index (14.72 MJ/m3/MPa) of the MC-OPG with AA/FA ratio of 0.20 were the lowest. The outcome of this study supports the utilisation of Na2CO3 to partially substitute Na2SiO3 for the development of OPGs.
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autor
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Chemical Engineering Technology, 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Chemical Engineering Technology, 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Chemical Engineering Technology, 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Chemical Engineering Technology, 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Chemical Engineering Technology, 01000 Perlis, Malaysia
autor
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Mechanical Engineering Technology, 02600 Arau, Perlis, Malaysia
autor
  • Universiti Malaysia Perlis (UniMAP), Geopolymer and Green Technology, Centre of Excellence (CEGeoGTech), 01000 Perlis, Malaysia
  • Universiti Malaysia Perlis (UniMAP), Faculty of Chemical Engineering Technology, 01000 Perlis, Malaysia
Bibliografia
  • [1] N.B. Singh, Minerals 8 (7), 299 (2018).
  • [2] K. Naupane, Clean. Mater. 6, 100138 (2022).
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  • [5] C. Ma, B. Zhao, S. Guo, G. Long, Y. Xie, J. Clean. Prod. 220, 188-199 (2019).
  • [6] B. Nematollahi, J. Sanjayan, F.U.A. Shaikh, Ceram. Int. 41 (4), 5696-5704 (2015).
  • [7] A. Adesina, Environ. Dev. Sustain., 100016 (2021).
  • [8] N. Hui-Teng, H. Cheng-Yong, L. Yun-Ming, M.M.A.B. Abdullah, K.E. Hun, H.M. Razi, N. Yong-Sing, J. Mater. Res. Technol. 12, 1212-1226 (2021).
  • [9] M. Dong, M. Elchalakani, A. Karrech, Constr. Build. Mater. 236, 117611 (2020).
  • [10] J. Yu, H.-L. Wu, C.K. Leung, J. Clean. Prod. 262, 121343 (2020).
  • [11] B.J. Mathew, M. Sudhakar, C. Natarajan, Int. J. Comput. Eng. Res. 3 (1), 207-212 (2013).
  • [12] R. Xiao, Y. Ma, X. Jiang, M. Zhang, Y. Zhang, Y. Wang, B. Huang, Q. He, J. Clean. Prod. 252, 119610 (2020).
  • [13] T. Yang, Z. Zhang, F. Zhang, Y. Gao, Q. Wu, J. Clean. Prod. 253, 120047 (2020).
  • [14] W-J. Long, X-W. Tan, B-X. Han, N-X. Han, F. Xing, J. Clean. Prod. 213, 406-414 (2019).
  • [15] S.F.A. Shah, B. Chen, M.R. Ahmad, M.A. Haque, J. Clean. Prod. 291, 125241 (2021).
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Uwagi
The author would like to acknowledge the Ministry of Higher Education, Malaysia, for providing the support (FRGS/1/2020/TK01/UNIMAP/02/2)
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-169f48c7-4b25-424e-b03c-973f130bfb63
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