Development of Renewable Material Hydrochar-Based CaAl Layered Double Hydroxide to Overcome Methyl Red Dyes Contaminant

• Autorzy: Mohadi Risfidian , Juleanti Novie , Palapa Neza Rahayu , Hidayati Nurlisa , Lesbani Aldes

Identyfikatory

DOI

10.12911/22998993/145541

• Języki publikacji: EN

Abstrakty

EN

The preparation of the CaAl/HC composite was carried out with a supporting material in the form of hydrochar from duku skin. The success of the preparation was demonstrated by XRD, FT-IR, and BET analysis. The diffractogram of CaAl/HC showed diffraction peaks at 2θ = 10.16° (003), 18.0° (002), 20.15° (006) and 65.4° (110). The diffraction showed similarity to diffraction in CaAl and hydrochar double layer hydroxyl. The FT-IR spectrum of CaAl/HC also showed similarity to the CaAl/HC double layer hydroxyl at 3448, 1635, and 1381 cm^-1. The characteristic spectrum of the hydrochar also appeared in CaAl/HC at 20.15. BET analysis showed an increase in the surface area of CaAl/HC before modification of 11.842 m²/g and increased to 22.635 m²/g of CaAl/HC. The ability of CaAl/HC as an adsorbent is determined through several parameters including selectivity, regeneration, isotherm, and thermodynamics. The results of dye selectivity showed that CaAl/HC was more likely to absorb MR dyes in a mixture of dyes (DG, MO, PR, MR, CR, and DR). The regeneration results showed the ability of CaAl/HC which lasted up to 73.26% in the fifth cycle.

Słowa kluczowe

EN

Ca/Al; layered double hydroxide; hydrochar; methyl red; selectivity

• Wydawca: Polskie Towarzystwo Inżynierii Ekologicznej ; Lublin University of Technology
• Czasopismo: Journal of Ecological Engineering
• Rocznik: 2022
• Tom: Vol. 23, nr 3
• Strony: 17--25
• Opis fizyczny: Bibliogr. 28 poz., rys., tab.

Twórcy

autor

Mohadi Risfidian

• Graduate School, Faculty of Mathematics and Natural Sciences, Sriwijaya University, Jl. Palembang-Prabumulih, Km. 90-32, Ogan Ilir, South Sumatra, Indonesia

autor

Juleanti Novie

• Magister Programme, Faculty of Mathematics and Natural Sciences, Sriwijaya University, Jl. Padang Selasa No. 524 Ilir Barat 1, Palembang, 30139, South Sumatra, Indonesia
• Research Center of Inorganic Materials and Complexes, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl.Padang Selasa Bukit Besar Palembang 30139, South Sumatera, Indonesia

• https://orcid.org/0000-0002-3334-4139

autor

Palapa Neza Rahayu

• Graduate School, Faculty of Mathematics and Natural Sciences, Sriwijaya University, Jl. Palembang-Prabumulih, Km. 90-32, Ogan Ilir, South Sumatra, Indonesia
• Research Center of Inorganic Materials and Complexes, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl.Padang Selasa Bukit Besar Palembang 30139, South Sumatera, Indonesia

autor

Hidayati Nurlisa

• Magister Programme, Faculty of Mathematics and Natural Sciences, Sriwijaya University, Jl. Padang Selasa No. 524 Ilir Barat 1, Palembang, 30139, South Sumatra, Indonesia

autor

Lesbani Aldes

• Graduate School, Faculty of Mathematics and Natural Sciences, Sriwijaya University, Jl. Palembang-Prabumulih, Km. 90-32, Ogan Ilir, South Sumatra, Indonesia
• Research Center of Inorganic Materials and Complexes, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl.Padang Selasa Bukit Besar Palembang 30139, South Sumatera, Indonesia

• https://orcid.org/0000-0001-5054-2324

Bibliografia

• 1. Arabpour A., Dan S., Hashemipour H. 2021. Preparation and Optimization of Novel Graphene Oxide and Adsorption Isotherm Study of Methylene Blue. Arabian Journal of Chemistry, 14(3), 103003. https://doi.org/10.1016/j.arabjc.2021.103003.
• 2. Badri A.F. et al. 2021. Mg-Al/Biochar Composite with Stable Structure for Malachite Green Adsorption from Aqueous Solutions. Bulletin of Chemical Reaction Engineering & Catalysis, 16(1), 149–160.
• 3. Bazan-Wozniak A., Pietrzak R. 2020. Adsorption of Organic and Inorganic Pollutants on Activated Bio-Carbons Prepared by Chemical Activation of Residues of Supercritical Extraction of Raw Plants. Chemical Engineering Journal, 393, 124785.
• 4. Dayanidhi K., Vadivel P., Jothi S., Eusuff N.S. 2020. Facile Synthesis of Silver@Eggshell Nanocomposite: A Heterogeneous Catalyst for The Removal of Heavy Metal Ions, Toxic Dyes and Microbial Contaminants from Water. Journal of Environmental Management 271, 110962. https://doi.org/10.1016/j.jenvman.2020.110962
• 5. Hashem A., Ahmad F., Badawy S.M. 2016. Adsorption of Direct Green 26 onto Fix 3500 Treated Sawdust: Equilibrium, Kinetic and Isotherms. Desalination and Water Treatment, 57(28), 13334–13346.
• 6. He H. et al. 2019. Efficient Phosphate Removal from Wastewater by MgAl-LDHs Modified Hydrochar Derived from Tobacco Stalk. Bioresource Technology Reports, 8, 100348. https://doi.org/10.1016/j.biteb.2019.100348
• 7. Hua P. et al. 2020. Adsorption of Acid Green and Procion Red on a Magnetic Geopolymer Based Adsorbent: Experiments, Characterization and Theoretical Treatment. Chemical Engineering Journal, 383.
• 8. Juleanti N. et al. 2021. The Capability of Biochar-Based CaAl and MgAl Composite Materials as Adsorbent for Removal Cr (VI) in Aqueous Solution. Science and Technology Indonesia, 6(3), 193–203.
• 9. Karri R.R., Tanzifi M., Yaraki M.T., Sahu J.N. 2018. Optimization and Modeling of Methyl Orange Adsorption onto Polyaniline Nano-Adsorbent through Response Surface Methodology and Differential Evolution Embedded Neural Network. Journal of Environmental Management 223, 517–529.
• 10. Luo X. et al. 2020. Hydrothermal Carbonization of Sewage Sludge and In-Situ Preparation of Hydrochar / MgAl-Layered Double Hydroxides Composites for Adsorption of Pb ( II ). Journal of Cleaner Production, 258, 120991. https://doi.org/10.1016/j.jclepro.2020.120991
• 11. Mahmoodi N.M., Jafar Abdi J., Bastani D. 2014. Direct Dyes Removal Using Modified Magnetic Ferrite Nanoparticle. Journal of Environmental Health Science and Engineering, 12(1), 1–10.
• 12. Milagres J.L. et al. 2017. Preparation and Evaluation of the Ca-Al Layered Double Hydroxide for Removal of Copper(II), Nickel(II), Zinc(II), Chromium(VI) and Phosphate from Aqueous Solutions. Journal of Environmental Chemical Engineering, 5(6), 5469–5480. http://dx.doi.org/10.1016/j.jece.2017.10.013.
• 13. Nazifa T.H. et al. 2018. Adsorption of Procion Red MX-5B and Crystal Violet Dyes from Aqueous Solution onto Corncob Activated Carbon. Journal of the Chinese Chemical Society, 65(2), 259–270.
• 14. Nazir M.A. et al. 2020. Surface Induced Growth of ZIF-67 at Co-Layered Double Hydroxide: Removal of Methylene Blue and Methyl Orange from Water. Applied Clay Science, 190, 105564. https://doi.org/10.1016/j.clay.2020.105564.
• 15. Normah et al. 2021. Competitive Removal of Cationic Dye Using Nial-Ldh Modified with Hydrochar.” Ecological Engineering and Environmental Technology, 22(4), 124–35.
• 16. Oktriyanti M., Palapa N.R., Mohadi R., Lesbani A. 2020. Effective Removal of Iron (II) from Aqueous Solution by Adsorption Using Zn/Cr Layered Double Hydroxides Intercalated with Keggin Ion. Journal of Ecological Engineering, 21(5), 63–71.
• 17. Onder A., Ilgin P., Ozay H., Ozay O. 2020. Removal of Dye from Aqueous Medium with PH-Sensitive Poly[(2-(Acryloyloxy)Ethyl]Trimethylammonium Chloride-Co-1-Vinyl-2-Pyrrolidone] Cationic Hydrogel. Journal of Environmental Chemical Engineering, 8(5), 104436. https://doi.org/10.1016/j.jece.2020.104436
• 18. Palapa N.R., Juleanti N., et al. 2020. Copper Aluminum Layered Double Hydroxide Modified by Biochar and Its Application as an Adsorbent for Procion Red. Journal of Water and Environment Technology, 18(6), 359–371.
• 19. Palapa N.R., Taher T., et al. 2020. CuAl LDH/Rice Husk Biochar Composite for Enhanced Adsorptive Removal of Cationic Dye from Aqueous Solution. Bulletin of Chemical Reaction Engineering & Catalysis, 15(2), 525–537.
• 20. Palapa N.R., Taher T., Wijaya A., Lesbani A. 2021. Modification of Cu / Cr Layered Double Hydroxide by Keggin Type Polyoxometalate as Adsorbent of Malachite Green from Aqueous Solution. Science and Technology Indonesia, 6(3), 209–217.
• 21. Pontes-Neto J.G. et al. 2019. Intercalation of Olanzapine into CaAl and NiAl Layered Double Hydroxides for Dissolution Rate Improvement: Synthesis, Characterization and in Vitro Toxicity. Journal of Drug Delivery Science and Technology, 52, 986–996. https://doi.org/10.1016/j.jddst.2019.05.034.
• 22. Siregar P.M.S.B.N., et al. 2021. Structural Stability of Ni/Al Layered Double Hydroxide Supported on Graphite and Biochar Toward Adorption of Congo Red. Science and Technology Indonesia, 6(2), 85–95.
• 23. Taher T. et al. 2020. A Comparative Study on Azo Dyes Removal Behavior to ZnAl and ZnCr LDHs. 9, 106–114.
• 24. Tran T.V., et al. 2020. Recyclable Fe3O4@C Nanocomposite as Potential Adsorbent for a Wide Range of Organic Dyes and Simulated Hospital Effluents. Environmental Technology and Innovation, 20, 101122. https://doi.org/10.1016/j.eti.2020.101122
• 25. Wahab N., et al. 2019. Synthesis, Characterization, and Applications of Silk/Bentonite Clay Composite for Heavy Metal Removal From Aqueous Solution. Frontiers in Chemistry 7, 1–12.
• 26. Wijaya A., et al. 2021. Innovative Modified of Cu-Al / C ( C = Biochar, Graphite ) Composites for Removal of Procion Red from Aqueous Solution, 6(4), 228–234.
• 27. Yu J., Zhang X., Wang D., Ping Li P. 2018. Adsorption of Methyl Orange Dye onto Biochar Adsorbent Prepared from Chicken Manure. Water Science and Technology, 77(5), 1303–1312.
• 28. Yuan Y., Yong X., Zhang H., Deng J. 2016. Biobased Microspheres Consisting of Poly(Trans-Anethole-Co-Maleic Anhydride) Prepared by Precipitation Polymerization and Adsorption Performance. ACS Sustainable Chemistry and Engineering, 4(3), 1446–1453.