PL EN


Preferencje help
Widoczny [Schowaj] Abstrakt
Liczba wyników
Tytuł artykułu

Obtaining and description of the MWCNTs-Pd nanocomposite

Wybrane pełne teksty z tego czasopisma
Identyfikatory
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
Purpose: The main aim of the research was to produce nanocomposites consisting of carbon nanotubes coated with palladium nanoparticles and the characterisation of the obtained materials. Design/methodology/approach: High quality multiwalled carbon nanotubes (MWCNTs) with the length of 100-400 nm and the diameter of 6-25 nm obtained in advance with Catalytic Chemical Vapour Deposition (CCVD) were employed in the investigations. Carbon nanotubes–palladium nanoparticles system was fabricated by direct deposition of palladium nanoparticles, produced earlier, onto the surface of multiwall carbon nanotubes. Findings: The investigations using transmission electron microscopy together with an EDS and XPS analysis have confirmed the fact of producing an MWCNTs-Pd nanocomposite. Examinations with Raman spectroscopy have allowed to determine the difference between the degree of defects of carbon nanotubes before and after modification with palladium nanoparticles. Research limitations/implications: The presence of palladium has influence on the electrical properties of the nanocomposite, enhances sensitivity and selectivity of the CNTsNPs system in contact with the chosen chemical substance, and the result is the changing of the conductivity of nanotubes. It is a basis for the application of the studied material as an active substance of sensors of chemical/biological compounds. Originality/value: The paper presents the results of investigations relating to the synthesis of a nanocomposite material consisting of multiwalled carbon nanotubes and Pd nanoparticles and the characteristics of the material produced in terms of its structure, morphology and the distribution of Pd nanoparticles on the external surface of multiwalled carbon nanotubes and chemical composition.
Rocznik
Strony
15--22
Opis fizyczny
Bibliogr. 13 poz.
Twórcy
  • Faculty of Mechanical Engineering, Silesian University of Technology, ul. Konarskiego 18A, 44-100 Gliwice, Poland
autor
  • Faculty of Mechanical Engineering, Silesian University of Technology, ul. Konarskiego 18A, 44-100 Gliwice, Poland
autor
  • Faculty of Mechanical Engineering, Silesian University of Technology, ul. Konarskiego 18A, 44-100 Gliwice, Poland
Bibliografia
  • [1] V. Georgakilas, D. Gournis, V. Tzitzios, L. Pasquato, D.M. Guldie, M. Prato, Decorating carbon nanotubes with metal or semiconductor nanoparticles, Journal of Materials Chemistry 17 (2007) 2679-2694.
  • [2] A.D. Dobrzańska-Danikiewicz, W. Wolany, G. Benke, Z. Rdzawski, The new MWCNTs rhenium nanocomposite, Physica Status Solidi B 251/12 (2014) 2485-2490.
  • [3] I. Stępińska, J. Radomska, M. Kozłowski, E. Czer wosz, W. Kowalski, K. Sobczak, Nanostructural films of CNTs covered with nanocrystals of palladium, Nanocontainers 1 (2014) 1–6.
  • [4] N. Karousis, G.E. Tsotsou, F. Evangelista, P. Rudolf, N. Ragoussis, N. Tagmatarchis, Carbon nanotubes decorated with palladium nanoparticles: synthesis, characterization, and catalytic activity, The Journal of Physical Chemistry C 112 (2008) 13463-13469.
  • [5] B. Wu, Y. Kuang, X. Zhang, J. Chen, Noble metal nanoparticles/carbon nanotubes nanohybrids: Synthesis and applications, Nano Today 6 (2011) 75-90.
  • [6] A.D. Dobrzańska-Danikiewicz, D. Łukowiec, Synthe sis and characterisation of Pt/MWCNTs nanocomposites, Physica Status Solidi (b) 250/12 (2013) 2569-2574.
  • [7] J.V. Rojas, C.H. Castano, Production of palladium nanoparticles supported on multiwalled carbon nanotubes by gamma irradiation, Radiation Physics and Chemistry 81 (2012) 16–21.
  • [8] H. Liu, L. Zhang, N. Wang, D. Sheng Su, Palladium Nanoparticles Embedded in the Inner Surfaces of Carbon Nanotubes: Synthesis, Catalytic Activity, and Sinter Resistance, Angewandte Chemie International Edition 53 (2014) 12634 -12638.
  • [9] F.P. Zamborini, S.M. Gross, R.W. Murray, Synthesis, Characterization, Reactivity, and Electrochemistry of Palladium Monolayer Protected Clusters, Langmuir 17 (2001) 481-488.
  • [10] M. Han, D. Jung, G.S. Lee, Palladium-nanoparticle-coated carbon nanotube gas sensor, Chemical Physics Letters 610–611 (2014) 261-266.
  • [11] R. Campesi, F. Cuevas, R. Gadiou, E. Leroy, M. Hirscher, C. Vix-Guterl, M. Latroche, Hydrogen storage properties of Pd nanoparticle/carbon template composites, Carbon 46 (2008) 206-214.
  • [12] A.D. Dobrzańska-Danikiewicz, D. Cichocki, M. Pawlyta, D. Łukowiec, W. Wolany, Synthesis conditions of carbon nanotubes with the chemical vapour deposition method, Physica Status Solidi (b) 251 (12) (2014) 2420-2425.
  • [13] X. Gu, W. Qi, X. Xu, Z. Sun, L. Zhang, W. Liu, X. Pan, D. Su. Covalently functionalized carbon nanotube supported Pd nanoparticles for catalytic reduction of 4-nitrophenol, Nanoscale 12 (2014) 6609-6616.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-10ad4c46-9898-4bf5-994a-24a80f094ab3
JavaScript jest wyłączony w Twojej przeglądarce internetowej. Włącz go, a następnie odśwież stronę, aby móc w pełni z niej korzystać.