Adsorption of Rhodamine B from water by activated char obtained from end-of-life tyre pyrolysis

• Autorzy: Kuśmierek Krzysztof , Świątkowski Andrzej , Kotkowski Tomasz , Cherbański Robert , Molga Eugeniusz

Identyfikatory

DOI

10.24425/cpe.2022.142290

• Języki publikacji: EN

Abstrakty

EN

Three activated chars obtained from end-of-life tyre pyrolysis differing in activation time (AC110 – 110 min, AC130 – 130 min, and AC150 – 150 min) were successfully used as adsorbents for the removal of model dye – Rhodamine B (RhB) from aqueous solutions. The effects of solution pH, adsorption kinetics, and equilibrium adsorption were investigated. The results showed that the adsorption was strongly pH-dependent; the highest percentage of RhB dye adsorbed was obtained at pH 2.0 and the removal efficiency decreased with an increase in solution pH. Adsorption kinetics was analyzed using pseudo-first-order, pseudo-second-order, Weber-Morris, and Boyd kinetic models. It was found that the pseudo-second-order kinetic equation was the most appropriate for describing the adsorption kinetics and that the RhB adsorption process was controlled by a film diffusion mechanism. Adsorption equilibrium data were fitted to the Langmuir, Freundlich, Temkin, and Elovich isotherm models. The equilibrium data were best represented by the Langmuir model with the monolayer adsorption capacities of 69.96, 94.34, and 133.3 μmol/g for AC110, AC130, and AC150, respectively. It was concluded that the adsorption of RhB was closely correlated with the specific surface area (and activation time) of the activated chars.

Słowa kluczowe

EN

Rhodamine B; adsorption; pyrolysis; waste tyres; tyre pyrolysis char

PL

Rodamina B; adsorpcja; piroliza; zużyte opony; zwęglenie pirolityczne opon

• Wydawca: Komitet Inżynierii Chemicznej i Procesowej Polskiej Akademii Nauk
• Czasopismo: Chemical and Process Engineering : New Frontiers
• Rocznik: 2023
• Tom: Vol. 44, nr 1
• Strony: art. no. e1
• Opis fizyczny: Bibliogr. 44 poz., tab., wykr.

Twórcy

autor

Kuśmierek Krzysztof

• Military University of Technology, Faculty of Advanced Technologies and Chemistry, ul. Kaliskiego 2, 00-908 Warsaw, Poland

• https://orcid.org/0000-0002-7948-8437

autor

Świątkowski Andrzej

• Military University of Technology, Faculty of Advanced Technologies and Chemistry, ul. Kaliskiego 2, 00-908 Warsaw, Poland

• https://orcid.org/0000-0002-6427-5439

autor

Kotkowski Tomasz

• Warsaw University of Technology, Faculty of Chemical and Process Engineering, ul. Waryńskiego 1, 00-645 Warsaw, Poland

• https://orcid.org/0000-0002-6018-0600

autor

Cherbański Robert

• Warsaw University of Technology, Faculty of Chemical and Process Engineering, ul. Waryńskiego 1, 00-645 Warsaw, Poland

• https://orcid.org/0000-0003-2649-7361

autor

Molga Eugeniusz

• Warsaw University of Technology, Faculty of Chemical and Process Engineering, ul. Waryńskiego 1, 00-645 Warsaw, Poland

• https://orcid.org/0000-0002-4788-3117

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Uwagi

Opracowanie rekordu ze środków MEiN, umowa nr SONP/SP/546092/2022 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2022-2023).