Polyoxometalate Intercalated Layered Double Hydroxide for Degradation of Procion Red

• Autorzy: Hanifah Yulizah , Mohadi Risfidian , Mardiyanto , Lesbani Aldes

Identyfikatory

DOI

10.12912/27197050/168088

• Języki publikacji: EN

Abstrakty

EN

The synthesis and characterization of layered double hydroxide (LDH) and intercalated polyoxometalate were presented.. The growth of polyoxometalate on Ni/Mg layered double hydroxide for degradation procion red (PR) was reported. The degradation parameters and organic dye removal efficiency of Zn/Mg-LDH and both composite LDH-polyoxometalate were determined by considering factors such as pH of dye solution, catalyst dosage, and time as variables of degradation. X-Ray, FTIR, and SEM spectroscopy confirmed the layered double hydroxide structure. XRD and FTIR analysis confirmed the single-phase of the as-made and polyoxometalate intercalated LDH. SEM images show the formation of aggregates of small various sizes. The catalytic activity of the material was evaluated in the degradation of PR as a model pollutant. The result showed that MgAl-SiW₁₂O₄₀ has a good degradation capacity for PR as compared to MgAl-PW₁₂O₄₀, ZnAl-SiW₁₂O₄₀, and ZnAl-PW₁₂O₄₀. The result shows that the LDH composite presents stability and has good photocatalytic activities toward the reduction of methylene blue. The materials utilized for the fifth regeneration are indicated by the FTIR results, which verified the LDH composite structure. The photodegradation process of procion red for immaculate ZnAl-LDH, MgAl-LDH, ZnAl-[PW₁₂O₄₀], ZnAl-[SiW₁₂O₄₀], MgAl-[PW₁₂O₄₀], MgAl-[SiW₁₂O₄₀] amounted to 68%, 70%, 56%, 79%, 74%, and 80%, respectively. The capacity of LDH-polyoxometalate composite material to successfully photodegrade, as measured by the percentage of degradation, revealed an increase in photodegradation catalysis and the ability of LDH to regenerate.

Słowa kluczowe

EN

polyoxometalate; LDH; layered double hydroxide; photocatalytic; methylene blue

• Wydawca: Lubelski Oddział Polskiego Towarzystwo Inżynierii Ekologicznej ; Lublin University of Technology ; WNGB Wydawnictwo Naukowe
• Czasopismo: Ecological Engineering & Environmental Technology
• Rocznik: 2023
• Tom: Vol. 24, iss. 6
• Strony: 109--116
• Opis fizyczny: Bibliogr. 22 poz., rys., tab.

Twórcy

autor

Hanifah Yulizah

• Graduate School of Mathematics and Natural Sciences, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl. Palembang Prabumulih Km.32 OganIlir 30662, Indonesia

• https://orcid.org/0000-0003-4152-5367

autor

Mohadi Risfidian

• Graduate School of Mathematics and Natural Sciences, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl. Palembang Prabumulih Km.32 OganIlir 30662, Indonesia
• Research Center of Inorganic Materials and Coordination Complexes, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl. Palembang Prabumulih Km.32 OganIlir 30662, Indonesia

• https://orcid.org/0000-0003-4974-4329

autor

Mardiyanto

• Department of Pharmacy, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl. Palembang Prabumulih Km.32 OganIlir 30662, Indonesia

• https://orcid.org/0000-0002-2951-4123

autor

Lesbani Aldes

• Graduate School of Mathematics and Natural Sciences, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl. Palembang Prabumulih Km.32 OganIlir 30662, Indonesia
• Research Center of Inorganic Materials and Coordination Complexes, Faculty of Mathematics and Natural Sciences, Universitas Sriwijaya, Jl. Palembang Prabumulih Km.32 OganIlir 30662, Indonesia

• https://orcid.org/0000-0001-5054-2324

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