Structure of aluminosilicate-supported nickel and iron oxides nanocomposites in gaseous and aqueous media

• Autorzy: Goncharuk Olena , Dyachenko Alla , Skwarek Ewa , Ischenko Olena , Andriyko Lyudmila , Borysenko Mykola , Sulym Iryna , Sternik Dariusz , Kowalska Klaudia , Marynin Andrii

Identyfikatory

DOI

10.37190/ppmp/144375

• Konferencja: Physicochemistry of interfaces - instrumental methods (22-26.08.2021 ; Lublin, Poland)
• Języki publikacji: EN

Abstrakty

EN

A series of mixed oxides was synthesized by deposition of a guest phase on a highly dispersed oxide matrix. Fumed nanooxides SiO₂, Al₂O₃, SiO₂/Al₂O₃, and SiO₂/Al₂O₃/TiO₂ with the specific surface area of 65-91 m²/g were selected as highly dispersed matrices. NiO/FexOy was deposited as a guest oxide using solvate-stimulated modification of a surface of fumed nanocarriers with nickel nitrate and iron(III) formate and subsequent heat treatment up to 600 °C to form NiO/FexOy. The aim of this work was to study the influence of the composition and structure of fumed oxide matrices and deposited guest phase on the behavior of the composites in gaseous and aqueous media using XRD, nitrogen adsorption and SEM/EDX, and quasi-elastic light scattering (QELS) methods. The lowtemperature nitrogen adsorption isotherms have a sigmoid shape with a narrow hysteresis loop characteristic of mesoporous materials. The specific surface area of composites varies from 65 to 120 m²/g. SEM data show denser aggregate structure of nanocomposites compared to the initial carriers. The primary particle size was in the 30-60 nm range. According to QELS data, there is a tendency to form aggregates of 100 nm - 10 µm in size in the aqueous media. The XRD method shows that the deposited metal oxides are in the form of crystalline phases of NiO with crystallites of 7-23 nm in size, but the iron oxide reflexes were not identified for NiO-containing composites.

Słowa kluczowe

EN

oxide nanocomposites; NiO/FexOy; textural properties; particle size distribution

• Wydawca: Oficyna Wydawnicza Politechniki Wrocławskiej
• Czasopismo: Physicochemical Problems of Mineral Processing
• Rocznik: 2022
• Tom: Vol. 58, iss. 2
• Strony: art. no. 144375
• Opis fizyczny: Bibliogr. 61 poz., rys., tab., wykr.

Twórcy

autor

Goncharuk Olena

• Chuiko Institute of Surface Chemistry, NASU, 17 General Naumov str., 03164 Kyiv, Ukraine
• Ovcharenko Institute of Biocolloidal Chemistry, NASU, 42 Vernadskii av., 03142 Kyiv, Ukraine
• National Technical University of Ukraine «Igor Sikorsky Kyiv Polytechnic Institute», 37 Peremohy av., 03056 Kyiv, Ukraine

• https://orcid.org/0000-0002-2554-8297

autor

Dyachenko Alla

• Taras Shevchenko National University of Kyiv, 64/13 Volodymyrs’ka str., 01033 Kyiv, Ukraine

• https://orcid.org/0000-0002-0955-5040

autor

Skwarek Ewa

• Chemistry Department, Maria Curie-Sklodowska University, M. Curie-Sklodowska sq. 3, 20031 Lublin, Poland

• https://orcid.org/0000-0003-4721-8704

autor

Ischenko Olena

• Taras Shevchenko National University of Kyiv, 64/13 Volodymyrs’ka str., 01033 Kyiv, Ukraine

autor

Andriyko Lyudmila

• Chuiko Institute of Surface Chemistry, NASU, 17 General Naumov str., 03164 Kyiv, Ukraine
• National University of Food Technology, 68 Volodymyrs’ka str., 01033 Kyiv, Ukraine

• https://orcid.org/0000-0001-5558-5374

autor

Borysenko Mykola

• Chuiko Institute of Surface Chemistry, NASU, 17 General Naumov str., 03164 Kyiv, Ukraine

• https://orcid.org/0000-0001-8707-1749

autor

Sulym Iryna

• Chuiko Institute of Surface Chemistry, NASU, 17 General Naumov str., 03164 Kyiv, Ukraine

• https://orcid.org/0000-0002-5012-885X

autor

Sternik Dariusz

• Chemistry Department, Maria Curie-Sklodowska University, M. Curie-Sklodowska sq. 3, 20031 Lublin, Poland

• https://orcid.org/0000-0002-3063-7542

autor

Kowalska Klaudia

• Chemistry Department, Maria Curie-Sklodowska University, M. Curie-Sklodowska sq. 3, 20031 Lublin, Poland

autor

Marynin Andrii

• National University of Food Technology, 68 Volodymyrs’ka str., 01033 Kyiv, Ukraine

• https://orcid.org/0000-0001-6692-7472

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Uwagi

Opracowanie rekordu ze środków MEiN, umowa nr SONP/SP/546092/2022 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2022-2023).