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2010 | 8 | 2 | 194-201
Tytuł artykułu

Photoacoustic spectroscopy for trace gas detection with cryogenic and room-temperature continuous-wave quantum cascade lasers

Treść / Zawartość
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The main characteristics that a sensor must possess for trace gas detection and pollution monitoring are high sensitivity, high selectivity and the capability to perform in situ measurements. The photacoustic Helmholtz sensor developed in Reims, used in conjunction with powerful Quantum Cascade Lasers (QCLs), fulfils all these requirements. The best cell response is # 1200 V W−1 cm and the corresponding ultimate sensitivity is j 3.3 × 10−10 W cm−11 Hz−11/2. This efficient sensor is used with mid-infrared QCLs from Alpes Lasers to reach the strong fundamental absorption bands of some atmospheric gases. A first cryogenic QCL emitting at 7.9 μm demonstrates the detection of methane in air with a detection limit of 3 ppb. A detection limit of 20 ppb of NO in air is demonstrated using another cryogenic QCL emitting in the 5.4 μm region. Real in-situ measurements can be achieved only with room-temperature QCLs. A room-temperature QCL emitting in the 7.9 μm region demonstrates the simultaneous detection of methane and nitrous oxide in air (17 and 7 ppb detection limit, respectively). All these reliable measurements allow the estimated detection limit for various atmospheric gases using quantum cascade lasers to be obtained. Each gas absorbing in the infrared may be detected at a detection limit in the ppb or low-ppb range.
Wydawca

Czasopismo
Rocznik
Tom
8
Numer
2
Strony
194-201
Opis fizyczny
Daty
wydano
2010-04-01
online
2010-01-30
Twórcy
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France, virginie.zeninari@univ-reims.fr
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France
autor
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France
  • Groupe de Spectrométrie Moléculaire et Atmosphérique, UMR CNRS 6089, UFR Sciences Exactes et Naturelles, Moulin de la Housse, BP 1039, 51687, Reims, Cedex 2, France
Bibliografia
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Typ dokumentu
Bibliografia
Identyfikatory
Identyfikator YADDA
bwmeta1.element.-psjd-doi-10_2478_s11534-009-0042-8
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