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2014 | 12 | 9 | 937-952
Tytuł artykułu

A multi-property fluorescent probe for the investigation of polymer dynamics near the glass transition

Treść / Zawartość
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
In addition to the commonly observed single molecule fluorescence intensity fluctuations due to molecular reorientation dynamics, a perylene bisimide-calixarene compound (1) shows additional on-off fluctuations due to its ability to undergo intramolecular excited state electron transfer (PET). This quenching process is turned on rather sharply when a film of poly(vinylacetate) containing 1 is heated above its glass transition temperature (T g), which indicates that the electron transfer process depends on the availability of sufficient free volume. Spatial heterogeneities cause different individual molecules to reach the electron transfer regime at different temperatures, but these heterogeneities also fluctuate in time: in the matrix above T g molecules that are mostly nonfluorescent due to PET can become fluorescent again on timescales of seconds to minutes. The two different mechanisms for intensity fluctuation, rotation and PET, thus far only observed in compound 1, make it a unique probe for the dynamics of supercooled liquids.
Słowa kluczowe
Wydawca

Czasopismo
Rocznik
Tom
12
Numer
9
Strony
937-952
Opis fizyczny
Daty
wydano
2014-09-01
online
2014-05-01
Twórcy
  • University of Amsterdam
  • Würzburg University
  • Würzburg University
  • University of Amsterdam
Bibliografia
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Identyfikator YADDA
bwmeta1.element.-psjd-doi-10_2478_s11532-014-0544-0
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