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Czasopismo
2014 | 12 | 2 | 164-172
Tytuł artykułu

Application of Box-Behnken design with response surface methodology for modeling and optimizing ultrasonic oxidation of arsenite with H2O2

Treść / Zawartość
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
A combined ultrasound (US)/H2O2 process was used to oxidize arsenite to arsenate, yielding a synergistic effect value of 1.26. This showed that the combined process could be an effective method of oxidizing arsenite, instead of using either ultrasonic or H2O2 oxidation processes. This combined process was successfully modeled and optimized using a Box-Behnken design with response surface methodology (RSM). The effects of the US power density, the initial concentration of arsenite, and the H2O2 concentration on the sonochemical oxidation efficiency of arsenite were investigated. Analysis of variance indicated that the proposed quadratic model successfully interpreted the experimental data with coefficients of determination of R 2 = 0.95 and adjusted R 2 = 0.91. Through this model, we can predict and control the oxidation efficiency under different conditions. Furthermore, the optimal conditions for the oxidation of arsenite were found to be a US power density of 233.26 W L−1, an initial arsenite concentration of 0.5 mg L−1, and an H2O2 concentration of 74.29 mg L−1. The predicted oxidation efficiency obtained from the RSM under the optimal conditions was 88.95%. A confirmation test of the optimal conditions verified the validity of the model, yielding an oxidation efficiency of 90.1%.
Wydawca

Czasopismo
Rocznik
Tom
12
Numer
2
Strony
164-172
Opis fizyczny
Daty
wydano
2014-02-01
online
2013-11-27
Twórcy
autor
  • Korea University
autor
  • Korea University
  • Korea University
autor
  • Korea University
autor
  • Kumoh National Institute of Technology
  • Korea University
autor
  • University of Malaya
Bibliografia
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Typ dokumentu
Bibliografia
Identyfikatory
Identyfikator YADDA
bwmeta1.element.-psjd-doi-10_2478_s11532-013-0360-y
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