Sn-Ni-Bi liquid phase thermodynamic properties

• Autorzy: Nikolina Milcheva , Jolanta Romanowska , Gueorgui Vassilev
• Języki publikacji: EN

Abstrakty

EN

Experimental data of bismuth activity coefficients at 1773 K were obtained by isopiestic method and compared to calculated values. Thermodynamic properties of the Sn-Ni-Bi liquid phase were estimated by means of the general solution model and by the methods of Kohler. Description of the ternary liquid phase (Gibbs excess energy dependence on the temperature and the composition) was achieved by using available thermodynamic data of the constitutive binary systems (Ni-Bi, Sn-Bi, Sn-Ni). A comparison between calculated quantities and experimental data wasconducted. The present assessment with thermodynamically optimized values of the system Sn-Ni-Bi (obtained by the CALPHAD approach) was in good agreement. The suggested appearance of a liquid phase miscibility gap at high temperatures is in agreement with the experimental bismuth activity data and with the assessed thermochemical functions. [...]

Słowa kluczowe

EN

Thermodynamics; General solution model; Ternary interaction parameters; Bi-Ni-Sn system; Bismuth activity coefficients

• Czasopismo: Open Chemistry
• Rocznik: 2011
• Tom: 9
• Numer: 1
• Strony: 149-156

Daty

wydano

2011-02-01

online

2010-12-16

Twórcy

autor

Nikolina Milcheva

• Faculty of Chemistry, University of Plovdiv, Plovdiv, Bulgaria

autor

Jolanta Romanowska

• Technical University of Rzeszow, Rzeszow, Poland

autor

Gueorgui Vassilev

• Faculty of Chemistry, University of Plovdiv, Plovdiv, Bulgaria,

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Identyfikatory

DOI

10.2478/s11532-010-0128-6