Czasopismo
Tytuł artykułu
Autorzy
Warianty tytułu
Języki publikacji
Abstrakty
Herein we demonstrate a method to improve the power conversion efficiency (PCE) parameter of organic photovoltaic (OPV) devices based on the electron acceptor N,N’-bis(1- ethylpropyl)-perylene-3,4,9,10-tetracarboxylic diimide (PDI) blended with the electron donor poly(indenofluorene)-aryloctyl (PIF-Aryl). The device parameters of the short-circuit current, open-circuit voltage and fill factor are found increased after the insertion of a thin poly [9, 9-dioctylfluorene-co-N- [4-(3-methylpropyl)]-diphenylamine] (TFB) photoactive interlayer between the hole-collecting electrode and the photoactive layer of the device. Unlike to most of the cases where interlayers serve as charge extractors, in our system the polymeric interlayer serves as a morphology modifying agent that drives the PDI component to segregate better at the interface with the device cathode; that is at the carrier-collecting electrode interface, which is not in physical contact with the interlayer. The processes of energy/charge transfer of the TFB excitons to/with the PIF-Aryl:PDI top-layer are also addressed. Charge transfer reactions dominate at the TFB/PIF-Aryl:PDI interface but no significant contribution in the photocurrent generation is seen in the photoaction spectra of the bilayer device.
Słowa kluczowe
Czasopismo
Rocznik
Tom
Strony
24-38
Opis fizyczny
Daty
otrzymano
2013-06-15
zaakceptowano
2013-07-17
online
2013-10-07
Twórcy
autor
-
Centre for Nanoscience and Technology@PoliMi,
Fondazione Istituto Italiano di Tecnologia,
Via Giovanni Pascoli 70/3, 20133 Milano, Italy
autor
-
Instituto Madrileno de Estudios Avanzados en Nanociencia
(IMDEA-Nanociencia), c/Faraday 9,
Cantoblanco, 28049, Madrid, Spain
autor
-
Centre for Nanoscience and Technology@PoliMi,
Fondazione Istituto Italiano di Tecnologia,
Via Giovanni Pascoli 70/3, 20133 Milano, Italy
autor
-
Instituto Madrileno de Estudios Avanzados en Nanociencia
(IMDEA-Nanociencia), c/Faraday 9,
Cantoblanco, 28049, Madrid, Spain
autor
-
Department of Chemistry ”G. Ciamician” University of Bologna,
Via Selmi 2, 40126 Bologna, Italy
autor
-
Centre for Nanoscience and Technology@PoliMi,
Fondazione Istituto Italiano di Tecnologia,
Via Giovanni Pascoli 70/3, 20133 Milano, Italy -
Department of Chemistry ”G. Ciamician” University of Bologna,
Via Selmi 2, 40126 Bologna, Italy
autor
-
Max-Planck Institute for Polymer Research, Ackermannweg 10,
D-55128, Mainz, Germany
autor
-
Centre for Polymer Science & Engineering,
Indian Institute of Technology Delhi, New Delhi 110016, India
autor
-
Centre for Nanoscience and Technology@PoliMi,
Fondazione Istituto Italiano di Tecnologia,
Via Giovanni Pascoli 70/3, 20133 Milano, Italy, pekeivan@iit.it
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Typ dokumentu
Bibliografia
Identyfikatory
Identyfikator YADDA
bwmeta1.element.-psjd-doi-10_2478_oph-2013-0003