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2013 | 1 | 24-38
Tytuł artykułu

Improving the layer morphology of solution-processed perylene diimide organic solar cells with the use of a polymeric interlayer

Treść / Zawartość
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
Herein we demonstrate a method to improve the power conversion efficiency (PCE) parameter of organic photovoltaic (OPV) devices based on the electron acceptor N,N’-bis(1- ethylpropyl)-perylene-3,4,9,10-tetracarboxylic diimide (PDI) blended with the electron donor poly(indenofluorene)-aryloctyl (PIF-Aryl). The device parameters of the short-circuit current, open-circuit voltage and fill factor are found increased after the insertion of a thin poly [9, 9-dioctylfluorene-co-N- [4-(3-methylpropyl)]-diphenylamine] (TFB) photoactive interlayer between the hole-collecting electrode and the photoactive layer of the device. Unlike to most of the cases where interlayers serve as charge extractors, in our system the polymeric interlayer serves as a morphology modifying agent that drives the PDI component to segregate better at the interface with the device cathode; that is at the carrier-collecting electrode interface, which is not in physical contact with the interlayer. The processes of energy/charge transfer of the TFB excitons to/with the PIF-Aryl:PDI top-layer are also addressed. Charge transfer reactions dominate at the TFB/PIF-Aryl:PDI interface but no significant contribution in the photocurrent generation is seen in the photoaction spectra of the bilayer device.
Słowa kluczowe
Wydawca

Rocznik
Tom
1
Strony
24-38
Opis fizyczny
Daty
otrzymano
2013-06-15
zaakceptowano
2013-07-17
online
2013-10-07
Twórcy
autor
  • Centre for Nanoscience and Technology@PoliMi,
    Fondazione Istituto Italiano di Tecnologia,
    Via Giovanni Pascoli 70/3, 20133 Milano, Italy
  • Instituto Madrileno de Estudios Avanzados en Nanociencia
    (IMDEA-Nanociencia), c/Faraday 9,
    Cantoblanco, 28049, Madrid, Spain
  • Centre for Nanoscience and Technology@PoliMi,
    Fondazione Istituto Italiano di Tecnologia,
    Via Giovanni Pascoli 70/3, 20133 Milano, Italy
  • Instituto Madrileno de Estudios Avanzados en Nanociencia
    (IMDEA-Nanociencia), c/Faraday 9,
    Cantoblanco, 28049, Madrid, Spain
  • Department of Chemistry ”G. Ciamician” University of Bologna,
    Via Selmi 2, 40126 Bologna, Italy
  • Centre for Nanoscience and Technology@PoliMi,
    Fondazione Istituto Italiano di Tecnologia,
    Via Giovanni Pascoli 70/3, 20133 Milano, Italy
  • Department of Chemistry ”G. Ciamician” University of Bologna,
    Via Selmi 2, 40126 Bologna, Italy
  • Max-Planck Institute for Polymer Research, Ackermannweg 10,
    D-55128, Mainz, Germany
  • Centre for Polymer Science & Engineering,
    Indian Institute of Technology Delhi, New Delhi 110016, India
  • Centre for Nanoscience and Technology@PoliMi,
    Fondazione Istituto Italiano di Tecnologia,
    Via Giovanni Pascoli 70/3, 20133 Milano, Italy, pekeivan@iit.it
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Typ dokumentu
Bibliografia
Identyfikatory
Identyfikator YADDA
bwmeta1.element.-psjd-doi-10_2478_oph-2013-0003
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